Laboratory-scale X-ray absorption spectroscopy approach for actinide research Experiment at the uranium L3-edge

التفاصيل البيبلوغرافية
العنوان: Laboratory-scale X-ray absorption spectroscopy approach for actinide research Experiment at the uranium L3-edge
المؤلفون: René Bes, Simo Huotari, Greg Leinders, Janne Pakarinen, Kristina O. Kvashnina, Ari-Pekka Honkanen, Taru Ahopelto
المساهمون: Department of Physics, Helsinki In Vivo Animal Imaging Platform (HAIP)
المصدر: Journal of Nuclear Materials 507(2018), 50-53
سنة النشر: 2018
مصطلحات موضوعية: Nuclear and High Energy Physics, Absorption spectroscopy, Nuclear engineering, chemistry.chemical_element, 01 natural sciences, 7. Clean energy, 114 Physical sciences, 010305 fluids & plasmas, law.invention, law, EXAFS SPECTROMETER, 0103 physical sciences, General Materials Science, FACILITY, Crystal optics, SPECIATION, 010302 applied physics, X-ray absorption spectroscopy, Nuclear fuel, ta114, Actinide, Uranium, Synchrotron, STATE, Nuclear Energy and Engineering, chemistry, Beamline, 13. Climate action, BEAMLINE, CRYSTAL SPECTROMETER, SYSTEM, FINE-STRUCTURE
الوصف: We report the first proof of principle of an efficient and cost-effective bentchtop alternatives to synchrotron radiation beamlines to perform at laboratory scale Xray Absorption Spectroscopy (XAS) at the U L3-edge in transmission mode. We find excellent agreement with synchrotron-based studies for concentrated samples, in reasonable acquisition time, for UO2, KUO3 and b-UO3 samples. The approach described here already constitutes an inexpensive answer to the XAS beamline over-subscription in the field of actinide’s research for state of the art experiments. Moreover, our results opens the door to many future applications in the field of actinide’s research, including f-electron chemistry, environmental chemistry and nuclear energy physico-chemistry such as advanced nuclear fuel and long term nuclear waste disposal.
وصف الملف: application/pdf
اللغة: English
تدمد: 0022-3115
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::191d06e269addd15b2f642b759958529
https://doi.org/10.1016/j.jnucmat.2018.04.034
حقوق: OPEN
رقم الأكسشن: edsair.doi.dedup.....191d06e269addd15b2f642b759958529
قاعدة البيانات: OpenAIRE