Detoxification of highly acidic hemicellulosic hydrolysate from wheat straw by diananofiltration with a focus on phenolic compounds
العنوان: | Detoxification of highly acidic hemicellulosic hydrolysate from wheat straw by diananofiltration with a focus on phenolic compounds |
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المؤلفون: | Andreia R. S. Teixeira, Marie-Laure Lameloise, Marielle Bouix, Axel Fayet, Florent Allais |
المساهمون: | Agro-Biotechnologies Industrielles (ABI), AgroParisTech, Université Paris Saclay (COmUE), Génie et Microbiologie des Procédés Alimentaires (GMPA), Institut National de la Recherche Agronomique (INRA)-AgroParisTech, Ingénierie, Procédés, Aliments (GENIAL), Region Grand Est, Conseil Departemental de la Marne and Grand Reims |
المصدر: | Journal of Membrane Science Journal of Membrane Science, Elsevier, 2018, 566, pp.112-121. ⟨10.1016/j.memsci.2018.08.045⟩ |
بيانات النشر: | HAL CCSD, 2018. |
سنة النشر: | 2018 |
مصطلحات موضوعية: | [SDV]Life Sciences [q-bio], Filtration and Separation, 02 engineering and technology, 010501 environmental sciences, Furfural, 01 natural sciences, Biochemistry, Diafiltration, Hydrolysate, Acetic acid, chemistry.chemical_compound, Hemicellulosic hydrolysate, [SDV.IDA]Life Sciences [q-bio]/Food engineering, Osmotic pressure, General Materials Science, [SPI.GPROC]Engineering Sciences [physics]/Chemical and Process Engineering, Physical and Theoretical Chemistry, 0105 earth and related environmental sciences, Steam explosion, Chromatography, food and beverages, Sulfuric acid, Straw, 021001 nanoscience & nanotechnology, Nanofiltration, Phenolic compounds, chemistry, 0210 nano-technology, Detoxification |
الوصف: | International audience; Nanofiltration was studied for detoxification of lignocellulose hydrolysates obtained in harsh conditions. A hemicellulosic hydrolysate obtained from sulfuric acid steam explosion of wheat straw and presenting very low pH ( = 1) and high osmotic pressure (28 bar) was studied and 8 inhibitory compounds were followed, among which 4 phenolic compounds. Several polymeric nanofiltration membranes were compared for separation performances and permeabilities; DK membrane (GE Osmonics) proved suitable with high rejection of sugars ( > 99%) and lower rejections of inhibitors. Acetic acid and furfural were quasi-fully transmitted whereas the rejection of compounds ranked as follow: HMF (5-hydroxymethyl-furfural) < coumaric acid < levulinic acid < vanillin < ferulic acid < syringaldehyde with values of 40%, 50%, 60%, 80%, 90% and 98%, respectively, at a permeate flux of 14 L h(-1) m(-2). Diafiltration was carried out at a transmembrane pressure of 26 bar until 3 DV (Diafiltration Volume) to complete detoxification, and continuous and sequential-dilution modes were compared. Thanks to the permeability of the membrane to the monovalent form of sulfuric acid HSO4-, effective transmembrane pressure was increased and pH reached 2. At 3 DV, both modes showed removal performances between 92% (acetic acid and furfural) and 25% (syringaldehyde). Irreversible fouling was observed, leading to 30% permeability loss after diafiltration. |
اللغة: | English |
تدمد: | 0376-7388 |
URL الوصول: | https://explore.openaire.eu/search/publication?articleId=doi_dedup___::28843cc940f25ba14e1fbc62a77d3874 https://hal.inrae.fr/hal-02626386 |
حقوق: | CLOSED |
رقم الأكسشن: | edsair.doi.dedup.....28843cc940f25ba14e1fbc62a77d3874 |
قاعدة البيانات: | OpenAIRE |
تدمد: | 03767388 |
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