X-ray multi-probe data acquisition: A novel technique for laser pump x-ray transient absorption spectroscopy
| العنوان: | X-ray multi-probe data acquisition: A novel technique for laser pump x-ray transient absorption spectroscopy |
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| المؤلفون: | Anne Marie March, C. Kurtz, Lin X. Chen, Guy Jennings, Eli D. Kinigstein, Xiaobing Zuo, Klaus Attenkofer, Xiaoyi Zhang |
| المصدر: | Review of Scientific Instruments. 92:085109 |
| بيانات النشر: | AIP Publishing, 2021. |
| سنة النشر: | 2021 |
| مصطلحات موضوعية: | Materials science, Absorption spectroscopy, business.industry, Laser pumping, Laser, Signal, Photon counting, law.invention, Data acquisition, Optics, law, Ultrafast laser spectroscopy, Absorption (electromagnetic radiation), business, Instrumentation |
| الوصف: | We report the development and implementation of a novel data acquisition (DAQ) technique for synchrotron-based laser pump X-ray Transient Absorption (XTA) spectroscopy, called X-ray Multi-Probe DAQ (XMP DAQ). This technique utilizes high performance analog to digital converters and home-built software to efficiently measure and process the XTA signal from all x-ray pulses between laser excitations. XMP DAQ generates a set of time resolved x-ray absorption spectra at thousands of different pump-probe time delays simultaneously. Two distinct XMP DAQ schemes are deployed to accommodate different synchrotron storage ring filling patterns. Current Integration (CI) DAQ is a quasi-analog technique that implements a fitting procedure to extract the time resolved absorption intensity from the averaged fluorescence detector response. The fitting procedure eliminates issues associated with small drifts in the voltage baseline and greatly enhances the accuracy of the technique. Photon Counting (PC) DAQ is a binary technique that uses a time resolved histogram to calculate the XTA spectrum. While PC DAQ is suited to measure XTA data with closely spaced x-ray pulses (∼10 ns) and a low count rate (1 detected photon/pulse), CI DAQ works best for widely spaced pulses (tens of ns or greater) with a high count rate (1 detected photon/pulse). XMP DAQ produces a two-dimensional XTA dataset, enabling efficient quantitative analysis of photophysical and photochemical processes from the sub-nanosecond timescale to 100 μs and longer. |
| تدمد: | 1089-7623 0034-6748 |
| URL الوصول: | https://explore.openaire.eu/search/publication?articleId=doi_dedup___::561fa2f4f13e94dfe32f67c11e8ec5dd https://doi.org/10.1063/5.0050713 |
| رقم الأكسشن: | edsair.doi.dedup.....561fa2f4f13e94dfe32f67c11e8ec5dd |
| قاعدة البيانات: | OpenAIRE |
Find this article in full text from Scitation. | تدمد: | 10897623 00346748 |
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