Precise Determination of Blackbody Radiation Shifts in a Strontium Molecular Lattice Clock
العنوان: | Precise Determination of Blackbody Radiation Shifts in a Strontium Molecular Lattice Clock |
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المؤلفون: | Iritani, B., Tiberi, E., Skomorowski, W., Moszynski, R., Borkowski, M., Zelevinsky, T. |
سنة النشر: | 2023 |
مصطلحات موضوعية: | Chemical Physics (physics.chem-ph), Atomic Physics (physics.atom-ph), Physics - Chemical Physics, FOS: Physical sciences, Physics - Atomic and Molecular Clusters, Atomic and Molecular Clusters (physics.atm-clus), Physics - Atomic Physics |
الوصف: | Molecular lattice clocks enable the search for new physics, such as fifth forces or temporal variations of fundamental constants, in a manner complementary to atomic clocks. Blackbody radiation (BBR) is a major contributor to the systematic error budget of conventional atomic clocks and is notoriously difficult to characterize and control. Here, we combine infrared Stark-shift spectroscopy in a molecular lattice clock and modern quantum chemistry methods to characterize the polarizabilities of the Sr$_2$ molecule from dc to infrared. Using this description, we determine the static and dynamic blackbody radiation shifts for all possible vibrational clock transitions to the $10^{-16}$ level. This constitutes an important step towards mHz-level molecular spectroscopy in Sr$_2$, and provides a framework for evaluating BBR shifts in other homonuclear molecules. 6 pages, 4 figures, updated references |
اللغة: | English |
URL الوصول: | https://explore.openaire.eu/search/publication?articleId=doi_dedup___::87d334af28bde56eabd68e54aaff257d http://arxiv.org/abs/2306.00981 |
حقوق: | OPEN |
رقم الأكسشن: | edsair.doi.dedup.....87d334af28bde56eabd68e54aaff257d |
قاعدة البيانات: | OpenAIRE |
الوصف غير متاح. |