Precise Determination of Blackbody Radiation Shifts in a Strontium Molecular Lattice Clock

التفاصيل البيبلوغرافية
العنوان: Precise Determination of Blackbody Radiation Shifts in a Strontium Molecular Lattice Clock
المؤلفون: Iritani, B., Tiberi, E., Skomorowski, W., Moszynski, R., Borkowski, M., Zelevinsky, T.
سنة النشر: 2023
مصطلحات موضوعية: Chemical Physics (physics.chem-ph), Atomic Physics (physics.atom-ph), Physics - Chemical Physics, FOS: Physical sciences, Physics - Atomic and Molecular Clusters, Atomic and Molecular Clusters (physics.atm-clus), Physics - Atomic Physics
الوصف: Molecular lattice clocks enable the search for new physics, such as fifth forces or temporal variations of fundamental constants, in a manner complementary to atomic clocks. Blackbody radiation (BBR) is a major contributor to the systematic error budget of conventional atomic clocks and is notoriously difficult to characterize and control. Here, we combine infrared Stark-shift spectroscopy in a molecular lattice clock and modern quantum chemistry methods to characterize the polarizabilities of the Sr$_2$ molecule from dc to infrared. Using this description, we determine the static and dynamic blackbody radiation shifts for all possible vibrational clock transitions to the $10^{-16}$ level. This constitutes an important step towards mHz-level molecular spectroscopy in Sr$_2$, and provides a framework for evaluating BBR shifts in other homonuclear molecules.
6 pages, 4 figures, updated references
اللغة: English
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::87d334af28bde56eabd68e54aaff257d
http://arxiv.org/abs/2306.00981
حقوق: OPEN
رقم الأكسشن: edsair.doi.dedup.....87d334af28bde56eabd68e54aaff257d
قاعدة البيانات: OpenAIRE