CO 2 absorption in a high efficiency silicon nitride mesh contactor

التفاصيل البيبلوغرافية
العنوان: CO 2 absorption in a high efficiency silicon nitride mesh contactor
المؤلفون: Asterios Gavriilidis, Achilleas Constantinou, S Barrass, F. Pronk, J. Shaw, D Wenn, T. Bril
المصدر: Chemical Engineering Journal. :766-771
بيانات النشر: Elsevier BV, 2012.
سنة النشر: 2012
مصطلحات موضوعية: Diethanolamine, Materials science, General Chemical Engineering, Membrane, Analytical chemistry, General Chemistry, Industrial and Manufacturing Engineering, Carbon dioxide absorption, Microreactor, chemistry.chemical_compound, Chemical engineering, chemistry, Silicon nitride, Microchannel, Sodium hydroxide, Phase (matter), Mass transfer, Chemical Sciences, Environmental Chemistry, Absorption (chemistry), Multiphase contactor, Natural Sciences, Contactor
الوصف: CO 2 absorption in sodium hydroxide and diethanolamine solutions was investigated in a silicon nitride mesh contactor. Mesh contactors allow two phases to come into direct contact with each other, for the purpose of mass transfer between them without dispersing one phase into the other. The 1 μm thick silicon nitride mesh, containing a high density of uniform 0.5 μm pores, facilitated the stabilization of the gas liquid interface at its pores. Experimental results were obtained for 2 M NaOH or 2 M DEA solutions and 20% vol. CO 2 /N 2 inlet concentrations, with a fixed inlet molar ratio CO 2 :NaOH of 0.4. Results showed that 23% of the CO 2 contained in the inlet stream was removed within 0.5 s experimental gas residence time. CO 2 removal efficiency was higher when NaOH was used for absorption as compared to DEA. Experiments were also conducted with different mesh/membrane contactors: a PTFE membrane (thickness 20 μm, pore size 0.5–5 μm), a Ni-25 mesh (thickness 25 μm, pore size 25 μm) and a Ni-5 mesh (thickness 5 μm, pore size 5 μm). The silicon nitride mesh demonstrated the best performance primarily due to its small thickness.
وصف الملف: pdf
تدمد: 1385-8947
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::881d3cbc63a63d5372724924a8d04461
https://doi.org/10.1016/j.cej.2012.07.059
حقوق: OPEN
رقم الأكسشن: edsair.doi.dedup.....881d3cbc63a63d5372724924a8d04461
قاعدة البيانات: OpenAIRE