Magnetic graphene enabled tunable microwave absorber via thermal control

التفاصيل البيبلوغرافية
العنوان: Magnetic graphene enabled tunable microwave absorber via thermal control
المؤلفون: Faxiang Qin, Huicai Wang, Diana Estevez, Fu Gj, Le Quan, Hua-Xin Peng, Yang Li
المصدر: Nanotechnology. 29:245706
بيانات النشر: IOP Publishing, 2018.
سنة النشر: 2018
مصطلحات موضوعية: Materials science, Annealing (metallurgy), Bioengineering, 02 engineering and technology, Dielectric, 010402 general chemistry, 01 natural sciences, law.invention, law, General Materials Science, Electrical and Electronic Engineering, Electrical impedance, business.industry, Graphene, Mechanical Engineering, Reflection loss, Doping, General Chemistry, 021001 nanoscience & nanotechnology, 0104 chemical sciences, Mechanics of Materials, Optoelectronics, Dielectric loss, 0210 nano-technology, business, Microwave
الوصف: By synthesizing nitrogen-doped graphene (NG) via a facile thermal annealing method, a fine control of the amount and location of doped nitrogen as well as the oxygen-containing functional groups is achieved with varying annealing temperature. The favorable magnetic properties have been achieved for N-doped rGO samples obtained at two temperatures of all NG samples, i.e., 500 °C and 900 °C with saturation magnetization of 0.63 emu g-1 and 0.67 emu g-1 at 2 K, respectively. This is attributed to the optimized competition of the N-doping and reduction process at 500 °C and the dominated reduction process at 900 °C. NG obtained at 300 °C affords the best overall absorbing performance: when the absorber thickness is 3.0 mm, the maximum absorption was -24.6 dB at 8.51 GHz, and the absorption bandwidth was 4.89 GHz (7.55-12.44 GHz) below -10 dB. It owes its large absorbing intensity to the good impedance match and significant dielectric loss. The broad absorption bandwidth benefits from local fluctuations of dielectric responses contributed by competing mechanisms. Despite the significant contribution from materials loss to the absorption, the one quarter-wavelength model is found to be responsible for the reflection loss peak positions. Of particular significance is that an appropriate set of electromagnetic parameters associated with reasonable reduction is readily accessible by convenient control of annealing temperature to modulate the microwave absorbing features of graphene. Thus, NG prepared by thermal annealing promises to be a highly efficient microwave absorbent.
تدمد: 1361-6528
0957-4484
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::bf08f677d55a9cf0a9b38dee300893e7
https://doi.org/10.1088/1361-6528/aabaae
حقوق: CLOSED
رقم الأكسشن: edsair.doi.dedup.....bf08f677d55a9cf0a9b38dee300893e7
قاعدة البيانات: OpenAIRE