Bimetallic selenides with various valence transitions and high theoretical capacities are extensively studied as anodes for sodium-ion-batteries (SIBs), but their huge volume changes and poor capacity retention limit their practicality. Herein, a facile and controllable strategy using a binary Ni-Co metal-organic framework (MOF) precursors followed by the selenization process, which produced a cobalt nickel selenide/N-doped carbon composite ((CoNi)Se