Toward Biodegradable Electronics: Ionic Diodes Based on a Cellulose Nanocrystal–Agarose Hydrogel
| العنوان: | Toward Biodegradable Electronics: Ionic Diodes Based on a Cellulose Nanocrystal–Agarose Hydrogel |
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| المؤلفون: | Francesco D'Acierno, Parisa Mehrkhodavandi, Jade Poisson, Zachary M. Hudson, Carl A. Michal, John D. W. Madden, Kudzanai Nyamayaro, Savvas G. Hatzikiriakos, Parya Keyvani |
| المصدر: | ACS Applied Materials & Interfaces. 12:52182-52191 |
| بيانات النشر: | American Chemical Society (ACS), 2020. |
| سنة النشر: | 2020 |
| مصطلحات موضوعية: | Materials science, Surface Properties, 01 natural sciences, 7. Clean energy, 010305 fluids & plasmas, chemistry.chemical_compound, 0103 physical sciences, General Materials Science, Cellulose, 010306 general physics, Dopant, Sepharose, Cationic polymerization, Hydrogels, Polyelectrolytes, Polyelectrolyte, Biodegradation, Environmental, chemistry, Chemical engineering, Nanocrystal, Self-healing hydrogels, Nanoparticles, Surface modification, Agarose, Electronics, Rheology |
| الوصف: | Bioderived cellulose nanocrystals (CNCs) are used to create light, flexible, biocompatible, and biodegradable electronic devices. Herein, surface modification of cellulose nanocrystals was employed to fabricate cationic and anionic CNCs. Subsequently, we demonstrated rectification behavior from a fixed junction between two agarose hydrogels doped with cationic and anionic cellulose nanocrystals. The current rectification ratio reaches 70 reproducibly, which is significantly higher than that for analogous diodes generated with microfibrillated cellulose (∼15) and the first polyelectrolyte gel diode (∼40). The current-voltage characteristics of the CNC-hydrogel diode are influenced by concentration, gel thickness, scanning frequency, and applied voltage. The high surface area of CNC resulted in high charge density after surface modification, which in turn resulted in good rectification behavior from only small amounts of dopant material. |
| تدمد: | 1944-8252 1944-8244 |
| URL الوصول: | https://explore.openaire.eu/search/publication?articleId=doi_dedup___::f53df5006a1aa77f2296cf5991e8422f https://doi.org/10.1021/acsami.0c15601 |
| حقوق: | CLOSED |
| رقم الأكسشن: | edsair.doi.dedup.....f53df5006a1aa77f2296cf5991e8422f |
| قاعدة البيانات: | OpenAIRE |
Find this issue from the American Chemical Society | تدمد: | 19448252 19448244 |
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