A New Type of Two-photon Forward Radiation in Pure Liquids

التفاصيل البيبلوغرافية
العنوان: A New Type of Two-photon Forward Radiation in Pure Liquids
المؤلفون: Bian, Hong-tao, Rao, Yi, Xu, Yan-yan, Liu, An-an, Guo, Yuan, Wang, Hong-fei
سنة النشر: 2007
المجموعة: Physics (Other)
مصطلحات موضوعية: Physics - Chemical Physics, Physics - Optics
الوصف: Unexpected spectral features are observed in the two photon spectrum of the pure water in the forward direction when an 80 femtosecond laser pulse is focused at 10^10Wcm-2 or less. Such intensity is much lower than the breakdown or stimulated threshold of the liquid water. The two broad features are about 2700cm-1 and 5000cm-1 red shifted from the hyper-Rayleigh wavelength, respectively, and they are quadratic with the laser intensity. They do not match the known Raman or hyper-Raman frequencies of water, and they are both centered at a narrow angle in the forward direction. Several other liquids also exhibited similar but molecular specific spectral features.
Comment: 4 pages, 4 figures
نوع الوثيقة: Working Paper
URL الوصول: http://arxiv.org/abs/0706.2408
رقم الأكسشن: edsarx.0706.2408
قاعدة البيانات: arXiv