Spin liquid in a single crystal of the frustrated diamond lattice antiferromagnet CoAl2O4

التفاصيل البيبلوغرافية
العنوان: Spin liquid in a single crystal of the frustrated diamond lattice antiferromagnet CoAl2O4
المؤلفون: Christensen, O. Zaharko. N. B., Cervellino, A., Tsurkan, V., Maljuk, A., Stuhr, U., Niedermayer, C., Yokaichiya, F., Argyriou, D. N., Boehm, M., Loidl, A.
المصدر: Physics Review B 84,094403(2011)
سنة النشر: 2011
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons
الوصف: We study spin liquid in the frustrated diamond lattice antiferromagnet CoAl2O4 by means of single crystal neutron scattering in zero and applied magnetic field. The magnetically ordered phase appearing below TN=8 K remains nonconventional down to 1.5 K. The magnetic Bragg peaks at the q=0 positions remain broad and their profiles have strong Lorentzian contribution. Additionally, they are connected by weak diffuse streaks along the <111> directions. These observations are explained within the spiral spin liquid model as short-range magnetic correlations of spirals populated at these finite temperatures, as the energy minimum around q=0 is flat and the energy of excited states with q=(111) is low. The agreement is only qualitative, leading us to suspect that microstructure effects are also important. Magnetic field significantly perturbs spin correlations. The 1.5 K static magnetic moment increases from 1.58 mB/Co at zero field to 2.08 mB/Co at 10 T, while the magnetic peaks, being still broad, acquire almost Gaussian profile. Spin excitations are rather conventional spin waves at zero field, resulting in the exchange parameters J1=0.92(1) meV, J2=0.101(2) meV and the anisotropy term D=-0.0089(2) meV for CoAl2O4. The application of a magnetic field leads to a pronounced broadening of the excitations at the zone center, which at 10 T appear gapless and nearly featureless.
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevB.84.094403
URL الوصول: http://arxiv.org/abs/1103.5799
رقم الأكسشن: edsarx.1103.5799
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevB.84.094403