Proximity-induced Shiba states in a molecular junction

التفاصيل البيبلوغرافية
العنوان: Proximity-induced Shiba states in a molecular junction
المؤلفون: Island, Joshua O., Gaudenzi, Rocco, de Bruijckere, Joeri, Burzuri, Enrique, Franco, Carlos, Mas-Torrent, Marta, Rovira, Concepcio, Veciana, Jaume, Klapwijk, Teun M., Aguado, Ramon, van der Zant, Herre S. J.
المصدر: Phys. Rev. Lett. 118, 117001 (2017)
سنة النشر: 2016
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Mesoscale and Nanoscale Physics, Condensed Matter - Superconductivity
الوصف: Superconductors containing magnetic impurities exhibit intriguing phenomena derived from the competition between Cooper pairing and Kondo screening. At the heart of this competition are the Yu-Shiba-Rusinov (Shiba) states which arise from the pair breaking effects a magnetic impurity has on a superconducting host. Hybrid superconductor-molecular junctions offer unique access to these states but the added complexity in fabricating such devices has kept their exploration to a minimum. Here, we report on the successful integration of a model spin 1/2 impurity, in the form of a neutral and stable all organic radical molecule, in proximity-induced superconducting break-junctions. Our measurements reveal excitations which are characteristic of a spin-induced Shiba state due to the radical's unpaired spin strongly coupled to a superconductor. By virtue of a variable molecule-electrode coupling, we access both the singlet and doublet ground states of the hybrid system which give rise to the doublet and singlet Shiba excited states, respectively. Our results show that Shiba states are a robust feature of the interaction between a paramagnetic impurity and a proximity-induced superconductor where the excited state is mediated by correlated electron-hole (Andreev) pairs instead of Cooper pairs.
Comment: 29 pages including supporting information
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevLett.118.117001
URL الوصول: http://arxiv.org/abs/1609.08316
رقم الأكسشن: edsarx.1609.08316
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevLett.118.117001