Spatio-temporal coherent control of thermal excitations in solids

التفاصيل البيبلوغرافية
العنوان: Spatio-temporal coherent control of thermal excitations in solids
المؤلفون: Sander, Mathias, Herzog, Marc, Pudell, Jan-Etienne, Bargheer, Matias, Weinkauf, Norbert, Pedersen, Martin, Newby, Gemma, Sellmann, Jan, Schwarzkopf, Jutta, Besse, Valentin, Temnov, Vasily, Gaal, Peter
المصدر: Phys. Rev. Lett. 119, 075901 (2017)
سنة النشر: 2017
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Materials Science
الوصف: X-ray reflectivity (XRR) measurements of femtosecond laser-induced transient gratings are applied to demonstrate the spatio-temporal coherent control of thermally induced surface deformations on ultrafast timescales. Using gracing incidence X-ray diffraction we unambiguously measure the amplitude of transient surface deformations with sub-\AA{} resolution. Understanding the dynamics of femtosecond TG excitations in terms of superposition of acoustic and thermal gratings makes it possible to develop new ways of coherent control in X-ray diffraction experiments. Being the dominant source of TG signal, the long-living thermal grating with spatial period $\Lambda$ can be canceled by a second, time-delayed TG excitation shifted by $\Lambda/2$. The ultimate speed limits of such an ultrafast X-ray shutter are inferred from the detailed analysis of thermal and acoustic dynamics in TG experiments.
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevLett.119.075901
URL الوصول: http://arxiv.org/abs/1704.01001
رقم الأكسشن: edsarx.1704.01001
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevLett.119.075901