Submolecular resolution by variation of IETS amplitude and its relation to AFM/STM signal

التفاصيل البيبلوغرافية
العنوان: Submolecular resolution by variation of IETS amplitude and its relation to AFM/STM signal
المؤلفون: de la Torre, Bruno, Švec, Martin, Foti, Giuseppe, Krejčí, Ondřej, Hapala, Prokop, Garcia-Lekue, Aran, Frederiksen, Thomas, Zbořil, Radek, Arnau, Andrés, Vázquez, Héctor, Jelínek, Pavel
المصدر: Phys. Rev. Lett. 119, 166001 (2017)
سنة النشر: 2017
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Materials Science
الوصف: Here we show scanning tunnelling microscopy (STM), non-contact atomic force microscopy (AFM) and inelastic electron tunnelling spectroscopy (IETS) measurements on organic molecule with a CO- terminated tip at 5K. The high-resolution contrast observed simultaneously in all channels unam- biguously demonstrates the common imaging mechanism in STM/AFM/IETS, related to the lateral bending of the CO-functionalized tip. The IETS spectroscopy reveals that the submolecular con- trast at 5K consists of both renormalization of vibrational frequency and variation of the amplitude of IETS signal. This finding is also corroborated by first principles simulations. We extend accord- ingly the probe-particle AFM/STM/IETS model to include these two main ingredients necessary to reproduce the high-resolution IETS contrast. We also employ the first principles simulations to get more insight into different response of frustrated translation and rotational modes of CO-tip during imaging.
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevLett.119.166001
URL الوصول: http://arxiv.org/abs/1710.06180
رقم الأكسشن: edsarx.1710.06180
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevLett.119.166001