Encapsulation Narrows Excitonic Homogeneous Linewidth of Exfoliated MoSe$_2$ Monolayer

التفاصيل البيبلوغرافية
العنوان: Encapsulation Narrows Excitonic Homogeneous Linewidth of Exfoliated MoSe$_2$ Monolayer
المؤلفون: Martin, Eric W., Horng, Jason, Ruth, Hanna G., Paik, Eunice, Wentzel, Michael-Henr, Deng, Hui, Cundiff, Steven T.
المصدر: Phys. Rev. Applied 14, 021002 (2020)
سنة النشر: 2018
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Materials Science
الوصف: The excitonic homogeneous linewidth of an exfoliated monolayer MoSe$_2$ encapsulated in hexagonal boron nitride is directly measured using multidimensional coherent spectroscopy with micron spatial resolution. The linewidth is 0.26 $\pm$ 0.02 meV, corresponding to a dephasing time $T_2 \approx$ 2.5 ps, which is almost half the narrowest reported values for non-encapsulated MoSe$_2$ flakes. We attribute the narrowed linewidth to Coulomb screening by the encapsulated material and suppression of non-radiative processes. Through direct measurements of encapsulated and non-encapsulated monolayers, we confirm that encapsulation reduces the sample inhomogeneity. However, linewidths measured using photoluminescence and linear absorption remain dominated by inhomogeneity, and these linewidths are roughly 5 times larger than the homogeneous linewidth in even the highest-quality encapsulated materials. The homogeneous linewidth of non-encapsulated monolayers is very sensitive to temperature cycling, whereas encapsulated samples are not modified by temperature cycling. The nonlinear signal intensity of non-encapsulated monolayers is degraded by high-power optical excitation, whereas encapsulated samples are very resilient to optical excitation with optical powers up to the point of completely bleaching the exciton.
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevApplied.14.021002
URL الوصول: http://arxiv.org/abs/1810.09834
رقم الأكسشن: edsarx.1810.09834
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevApplied.14.021002