Giant optical nonlinearity cancellation in quantum wells

التفاصيل البيبلوغرافية
العنوان: Giant optical nonlinearity cancellation in quantum wells
المؤلفون: Houver, S., Lebreton, A., Pereira, T. A. S., Xu, G., Colombelli, R., Kundu, I., Li, L. H., Linfield, E. H., Davies, A. G., Mangeney, J., Tignon, J., Ferreira, R., Dhillon, S. S.
سنة النشر: 2019
المجموعة: Condensed Matter
Physics (Other)
Quantum Physics
مصطلحات موضوعية: Physics - Optics, Condensed Matter - Other Condensed Matter, Quantum Physics
الوصف: Second-order optical nonlinearities can be greatly enhanced by orders of magnitude in resonantly excited nanostructures, theoretically predicted and experimentally investigated in a variety of semiconductor systems. These resonant nonlinearities continually attract attention, particularly in newly discovered materials, but tend not to be as efficient as currently predicted. This limits their exploitation in frequency conversion. Here, we present a clear-cut theoretical and experimental demonstration that the second-order nonlinear susceptibility can vary by orders of magnitude as a result of giant cancellation effects in systems with many confined quantum states. Using terahertz quantum cascade lasers as a model source to investigate interband and intersubband resonant nonlinearities, we show that these giant cancellations are a result of interfering second-order nonlinear contributions of light and heavy hole states. As well as of importance to understand and engineer the resonant optical properties of materials, this work can be employed as a new, extremely sensitive tool to elucidate the bandstructure properties of complex quantum well systems.
نوع الوثيقة: Working Paper
URL الوصول: http://arxiv.org/abs/1901.01033
رقم الأكسشن: edsarx.1901.01033
قاعدة البيانات: arXiv