Magnetic competition induced colossal magnetoresistance in n-type HgCr2Se4 under high pressures

التفاصيل البيبلوغرافية
العنوان: Magnetic competition induced colossal magnetoresistance in n-type HgCr2Se4 under high pressures
المؤلفون: Sun, J. P., Jiao, Y. Y., Yi, C. J., Dissanayake, S. E., Matsuda, M., Uwatoko, Y., Shi, Y. G., Li, Y. Q., Fang, Z., Cheng, J. -G.
المصدر: Phys. Rev. Lett. 123, 047201 (2019)
سنة النشر: 2019
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons
الوصف: The n-type HgCr2Se4 exhibits a sharp semiconductor-to-metal transition (SMT) in resistivity accompanying the ferromagnetic order at TC = 106 K. Here, we investigate the effects of pressure and magnetic field on the concomitant SMT and ferromagnetic order by measuring resistivity, dc and ac magnetic susceptibility, as well as single-crystal neutron diffraction under various pressures up to 8 GPa and magnetic fields up to 8 T. Our results demonstrate that the ferromagnetic metallic ground state of n-type HgCr2Se4 is destabilized and gradually replaced by an antiferromagnetic, most likely a spiral magnetic, and insulating ground state upon the application of high pressure. On the other hand, the application of external magnetic fields can restore the ferromagnetic metallic state again at high pressures, resulting in a colossal magnetoresistance (CMR) as high as ~ 3 * 10^11 % under 5 T and 2 K at 4 GPa. The present study demonstrates that n-type HgCr2Se4 is located at a peculiar critical point where the balance of competion between ferromagnetic and antiferromagnetic interactions can be easily tipped by the external stimuli, providing a new platform for achieving CMR in a single-valent system.
Comment: 6 pages, 4 figures
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevLett.123.047201
URL الوصول: http://arxiv.org/abs/1903.10689
رقم الأكسشن: edsarx.1903.10689
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevLett.123.047201