Nonlinear Spectroscopy and All-Optical Switching of Femtosecond Soliton Molecules

التفاصيل البيبلوغرافية
العنوان: Nonlinear Spectroscopy and All-Optical Switching of Femtosecond Soliton Molecules
المؤلفون: Kurtz, Felix, Ropers, Claus, Herink, Georg
سنة النشر: 2019
المجموعة: Nonlinear Sciences
Physics (Other)
مصطلحات موضوعية: Physics - Optics, Nonlinear Sciences - Pattern Formation and Solitons
الوصف: The emergence of confined structures and pattern formation are exceptional manifestations of concurring nonlinear interactions found in a variety of physical, chemical and biological systems[1]. Optical solitons are a hallmark of extreme spatial or temporal confinement enabled by a variety of nonlinearities. Such particle-like structures can assemble in complex stable arrangements, forming "soliton molecules"[2,3]. Recent works revealed oscillatory internal motions of these bound states, akin to molecular vibrations[4-8]. These observations beg the question as to how far the "molecular" analogy reaches, whether further concepts from molecular spectroscopy apply in this scenario, and if such intra-molecular dynamics can be externally driven or manipulated. Here, we probe and control such ultrashort bound-states in an optical oscillator, utilizing real-time spectroscopy and time-dependent external perturbations. We introduce two-dimensional spectroscopy of the linear and nonlinear bound-state response and resolve anharmonicities in the soliton interaction leading to overtone and sub-harmonic generation. Employing a non-perturbative interaction, we demonstrate all-optical switching between distinct states with different binding separation, opening up novel schemes of ultrafast spectroscopy, optical logic operations and all-optical memory.
Comment: 3 figures
نوع الوثيقة: Working Paper
DOI: 10.1038/s41566-019-0530-3
URL الوصول: http://arxiv.org/abs/1908.04323
رقم الأكسشن: edsarx.1908.04323
قاعدة البيانات: arXiv
الوصف
DOI:10.1038/s41566-019-0530-3