Nanoscale degeneracy lifting in a geometrically frustrated antiferromagnet

التفاصيل البيبلوغرافية
العنوان: Nanoscale degeneracy lifting in a geometrically frustrated antiferromagnet
المؤلفون: Frandsen, Benjamin A., Bozin, Emil S., Aza, Eleni, Martinez, Antonio Fernandez, Feygenson, Mikhail, Page, Katharine, Lappas, Alexandros
المصدر: Phys. Rev. B 101, 024423 (2020)
سنة النشر: 2020
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons
الوصف: The local atomic and magnetic structures of the compounds $A$MnO$_2$ ($A$ = Na, Cu), which realize a geometrically frustrated, spatially anisotropic triangular lattice of Mn spins, have been investigated by atomic and magnetic pair distribution function analysis of neutron total scattering data. Relief of frustration in CuMnO$_2$ is accompanied by a conventional cooperative symmetry-lowering lattice distortion driven by N\'eel order. In NaMnO$_2$, however, the distortion has a short-range nature. A cooperative interaction between the locally broken symmetry and short-range magnetic correlations lifts the magnetic degeneracy on a nanometer length scale, enabling long-range magnetic order in the Na-derivative. The degree of frustration, mediated by residual disorder, contributes to the rather differing pathways to a single, stable magnetic ground state in these two related compounds. This study demonstrates how nanoscale structural distortions that cause local-scale perturbations can lift the ground state degeneracy and trigger macroscopic magnetic order.
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevB.101.024423
URL الوصول: http://arxiv.org/abs/2001.09917
رقم الأكسشن: edsarx.2001.09917
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevB.101.024423