Correlating Nanocrystalline Structure with Electronic Properties in 2D Platinum Diselenide

التفاصيل البيبلوغرافية
العنوان: Correlating Nanocrystalline Structure with Electronic Properties in 2D Platinum Diselenide
المؤلفون: Lukas, Sebastian, Hartwig, Oliver, Prechtl, Maximilian, Capraro, Giovanna, Bolten, Jens, Meledin, Alexander, Mayer, Joachim, Neumaier, Daniel, Kataria, Satender, Duesberg, Georg S., Lemme, Max C.
المصدر: Advanced Functional Material, 2102929, 2021
سنة النشر: 2021
المجموعة: Condensed Matter
Physics (Other)
مصطلحات موضوعية: Condensed Matter - Materials Science, Physics - Applied Physics
الوصف: Platinum diselenide (PtSe${_2}$) is a two-dimensional (2D) material with outstanding electronic and piezoresistive properties. The material can be grown at low temperatures in a scalable manner which makes it extremely appealing for many potential electronics, photonics, and sensing applications. Here, we investigate the nanocrystalline structure of different PtSe${_2}$ thin films grown by thermally assisted conversion (TAC) and correlate them with their electronic and piezoresistive properties. We use scanning transmission electron microscopy for structural analysis, X-ray photoelectron spectroscopy (XPS) for chemical analysis, and Raman spectroscopy for phase identification. Electronic devices are fabricated using transferred PtSe${_2}$ films for electrical characterization and piezoresistive gauge factor measurements. The variations of crystallite size and their orientations are found to have a strong correlation with the electronic and piezoresistive properties of the films, especially the sheet resistivity and the effective charge carrier mobility. Our findings may pave the way for tuning and optimizing the properties of TAC-grown PtSe${_2}$ towards numerous applications.
نوع الوثيقة: Working Paper
DOI: 10.1002/adfm.202102929
URL الوصول: http://arxiv.org/abs/2104.03636
رقم الأكسشن: edsarx.2104.03636
قاعدة البيانات: arXiv