Energy-gap driven low-temperature magnetic and transport properties in Cr$_{1/3}M$S$_2$ ($M$ = Nb or Ta)

التفاصيل البيبلوغرافية
العنوان: Energy-gap driven low-temperature magnetic and transport properties in Cr$_{1/3}M$S$_2$ ($M$ = Nb or Ta)
المؤلفون: Hicken, T. J., Hawkhead, Z., Wilson, M. N., Huddart, B. M., Hall, A. E., Balakrishnan, G., Pratt, F. L., Clark, S. J., Lancaster, T.
سنة النشر: 2021
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons
الوصف: The helimagnets Cr$_{1/3}M$S$_2$ ($M$ = Nb or Ta) have attracted renewed attention due to the discovery of a chiral soliton lattice (CSL) stabilized in an applied magnetic field, but reports of unusual low-temperature transport and magnetic properties in this system lack a unifying explanation. Here we present electronic structure calculations that demonstrate the materials are half-metals. There is also a gap-like feature (width in range 40-100 meV) in the density of states of one spin channel. This electronic structure explains the low-temperature electronic and magnetic properties of Cr$_{1/3}M$S$_2$ ($M$ = Nb or Ta), with the gap-like feature particularly important for explaining the magnetic behavior. Our magnetometry measurements confirm the existence of this gap. Dynamic spin fluctuations driven by excitations across this gap are seen over a wide range of frequencies (0.1 Hz to MHz) with AC susceptibility and muon-spin relaxation ($\mu^+$SR) measurements. We show further how effects due to the CSL in Cr$_{1/3}$NbS$_2$, as detected with $\mu^+$SR, dominate over the gap-driven magnetism when the CSL is stabilized as the majority phase.
Comment: 6 pages, 4 figures
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevB.105.L060407
URL الوصول: http://arxiv.org/abs/2105.01393
رقم الأكسشن: edsarx.2105.01393
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevB.105.L060407