Third-order polarizability of interlayer excitons in hetero-bilayers

التفاصيل البيبلوغرافية
العنوان: Third-order polarizability of interlayer excitons in hetero-bilayers
المؤلفون: Quintela, M. F. C. Martins, Henriques, J. C. G., Peres, N. M. R.
المصدر: Phys. Rev. B 104, 205433 (2021)
سنة النشر: 2021
المجموعة: Condensed Matter
Quantum Physics
مصطلحات موضوعية: Condensed Matter - Mesoscale and Nanoscale Physics, Condensed Matter - Materials Science, Quantum Physics
الوصف: In this paper, we employ a fully microscopic approach to the study of interlayer excitons in hetero-bilayers. We use Fowler's and Karplus' method to access the dynamical polarizability of non--interacting interlayer excitons in a $\mathrm{WSe}_{2}/\mathrm{WS}_{2}$--based van der Waals heterostructure. Following from the calculation of the linear polarizability, we consider Svendsen's variational method to the calculation of the dynamic third--order polarizability. With this variational method, we study both two--photon absorption and third--harmonic generation processes for interlayer excitons in a $\mathrm{WSe}_{2}/\mathrm{WS}_{2}$ hetero--bilayer, discussing the various selection rules of intra--excitonic energy level transitions.
Comment: 13 pages, 7 figures
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevB.104.205433
URL الوصول: http://arxiv.org/abs/2106.11738
رقم الأكسشن: edsarx.2106.11738
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevB.104.205433