Deep-ultraviolet electroluminescence and photocurrent generation in graphene/hBN/graphene heterostructures

التفاصيل البيبلوغرافية
العنوان: Deep-ultraviolet electroluminescence and photocurrent generation in graphene/hBN/graphene heterostructures
المؤلفون: Song, Su-Beom, Yoon, Sangho, Kim, So Young, Yang, Sera, Seo, Seung-Young, Cha, Soonyoung, Jeong, Hyeon-Woo, Watanabe, Kenji, Taniguchi, Takashi, Lee, Gil-Ho, Kim, Jun Sung, Jo, Moon-Ho, Kim, Jonghwan
سنة النشر: 2021
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Materials Science, Condensed Matter - Mesoscale and Nanoscale Physics
الوصف: Hexagonal boron nitride (hBN) is a van der Waals semiconductor with a wide bandgap of ~ 5.96 eV. Despite the indirect bandgap characteristics of hBN, charge carriers excited by high energy electrons or photons efficiently emit luminescence at deep-ultraviolet (DUV) frequencies via strong electron-phonon interaction, suggesting potential DUV light emitting device applications. However, electroluminescence from hBN has not been demonstrated at DUV frequencies so far. In this study, we report DUV electroluminescence and photocurrent generation in graphene/hBN/graphene heterostructures at room temperature. Tunneling carrier injection from graphene electrodes into the band edges of hBN enables prominent electroluminescence at DUV frequencies. On the other hand, under DUV laser illumination and external bias voltage, graphene electrodes efficiently collect photo-excited carriers in hBN, which generates high photocurrent. Laser excitation micro-spectroscopy shows that the radiative recombination and photocarrier excitation processes in the heterostructures mainly originate from the pristine structure and the stacking faults in hBN. Our work provides a pathway toward efficient DUV light emitting and detection devices based on hBN.
Comment: 29 pages, 4 figures, Su-Beom Song and Sangho Yoon contributed equally to this work, To whom correspondence should be addressed: jonghwankim@postech.ac.kr
نوع الوثيقة: Working Paper
DOI: 10.1038/s41467-021-27524-w
URL الوصول: http://arxiv.org/abs/2112.00321
رقم الأكسشن: edsarx.2112.00321
قاعدة البيانات: arXiv
الوصف
DOI:10.1038/s41467-021-27524-w