Short-range Crystalline Order-Tuned Conductivity in Cr$_2$Si$_2$Te$_6$ van der Waals Magnetic Crystals

التفاصيل البيبلوغرافية
العنوان: Short-range Crystalline Order-Tuned Conductivity in Cr$_2$Si$_2$Te$_6$ van der Waals Magnetic Crystals
المؤلفون: Liu, Yu, Susilo, Resta A., Lee, Yongbin, Abeykoon, A. M. Milinda, Tong, Xiao, Hu, Zhixiang, Stavitski, Eli, Attenkofer, Klaus, Ke, Liqin, Chen, Bin, Petrovic, Cedomir
المصدر: ACS Nano 16, 13134 (2022)
سنة النشر: 2022
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons, Condensed Matter - Materials Science
الوصف: Two-dimensional magnetic materials (2DMM) are significant for studies on the nature of 2D long range magnetic order but also for future spintronic devices. Of particular interest are 2DMM where spins can be manipulated by electrical conduction. Whereas Cr$_2$Si$_2$Te$_6$ exhibits magnetic order in few-layer crystals, its large band gap inhibits electronic conduction. Here we show that the defect-induced short-range crystal order in Cr$_2$Si$_2$Te$_6$ on the length scale below 0.6 nm induces substantially reduced band gap and robust semiconducting behavior down to 2 K that turns to metallic above 10 GPa. Our results will be helpful to design conducting state in 2DMM and call for spin-resolved measurement of the electronic structure in exfoliated ultrathin crystals.
نوع الوثيقة: Working Paper
DOI: 10.1021/acsnano.2c06080
URL الوصول: http://arxiv.org/abs/2208.08648
رقم الأكسشن: edsarx.2208.08648
قاعدة البيانات: arXiv