Order-disorder Peierls instability in the kagome metal (Cs,Rb)V$_3$Sb$_5$

التفاصيل البيبلوغرافية
العنوان: Order-disorder Peierls instability in the kagome metal (Cs,Rb)V$_3$Sb$_5$
المؤلفون: Subires, D., Korshunov, A., Said, A. H., Sánchez, L., Ortiz, Brenden R., Wilson, Stephen D., Bosak, A., Blanco-Canosa, S.
سنة النشر: 2022
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons, Condensed Matter - Materials Science
الوصف: The nature of the charge density wave phases in the kagome metal compound AV$_3$Sb$_5$ has raised many questions and their origin is still under debate. Here, we combine diffuse scattering (DS) and inelastic x-ray scattering (IXS) to identify a 3-dimensional (3D) precursor of the charge order with propagation vector (0.5 0 0.5), which condenses into a 3D-CDW through a first order phase transition. The quasi-elastic critical scattering indicates that the dominant contribution to the diffuse precursor is the elastic central peak without phonon softening. However, the inelastic spectra show a small broadening of the Einstein-type phonon mode on approaching the phase transition. Our results point to the situation where the Fermi surface instability at the \textit{L} point is of order-disorder type with a critical growth of quasi-static domains. The results go beyond the classical weak-coupling Peierls transition dynamics and are discussed within models including strong-electron phonon coupling and non-adiabaticity.
نوع الوثيقة: Working Paper
DOI: 10.1038/s41467-023-36668-w
URL الوصول: http://arxiv.org/abs/2209.13342
رقم الأكسشن: edsarx.2209.13342
قاعدة البيانات: arXiv
الوصف
DOI:10.1038/s41467-023-36668-w