Entropy and Seebeck signals meet on the edges

التفاصيل البيبلوغرافية
العنوان: Entropy and Seebeck signals meet on the edges
المؤلفون: Cortés, Natalia, Vargas, Patricio, Ulloa, S. E.
سنة النشر: 2022
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Mesoscale and Nanoscale Physics
الوصف: We explore the electronic entropy per particle $s$ and Seebeck coefficient $\mathcal{S}$ in zigzag graphene ribbons. Pristine and edge-doped ribbons are considered using tight-binding models to inspect the role of edge states in the observed thermal transport properties. As a bandgap opens when the ribbons are doped at one or both edges, due to asymmetric edge potentials, we find that $s$ and $\mathcal{S}$ signals are closely related to each other: both develop sharp dip-peak lineshapes as the chemical potential lies in the gap, while the ratio $s/\mathcal{S}$ exhibits a near constant value equal to the elementary charge $e$ at low temperatures. This constant ratio suggests that $\mathcal{S}$ can be seen as the transport differential entropy per charge, as suggested by some authors. Our calculations also indicate that measurement of $s$ and $\mathcal{S}$ may be useful as a spectroscopic probe of different electronic energy scales involved in such quantities in gapped materials.
Comment: 6 pages, 6 figures
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevB.107.075433
URL الوصول: http://arxiv.org/abs/2210.00151
رقم الأكسشن: edsarx.2210.00151
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevB.107.075433