Dimensionality control and rotational symmetry breaking superconductivity in square-planar layered nickelates

التفاصيل البيبلوغرافية
العنوان: Dimensionality control and rotational symmetry breaking superconductivity in square-planar layered nickelates
المؤلفون: Chow, Lin Er, Rubi, Km, Yip, King Yau, Pierre, Mathieu, Leroux, Maxime, Liu, Xinyou, Luo, Zhaoyang, Zeng, Shengwei, Li, Changjian, Goiran, Michel, Harrison, Neil, Escoffier, Walter, Goh, Swee Kuan, Ariando, A.
سنة النشر: 2023
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Superconductivity, Condensed Matter - Materials Science, Condensed Matter - Strongly Correlated Electrons
الوصف: The interplay between dimensionality and various phases of matter is a central inquiry in condensed matter physics. New phases are often discovered through spontaneously broken symmetry. Understanding the dimensionality of superconductivity in the high-temperature cuprate analogue $-$ layered nickelates and revealing a new symmetry-breaking state are the keys to deciphering the underlying pairing mechanism. Here, we demonstrate the highly-tunable dimensionality and a broken rotational symmetry state in the superconductivity of square-planar layered nickelates. The superconducting state, probed by superconducting critical current and magnetoresistance within superconducting transition under direction-dependent in-plane magnetic fields, exhibits a $C_2$ rotational symmetry which breaks the $C_4$ rotational symmetry of the square-planar lattice. Furthermore, by performing detailed examination of the angular dependent upper critical fields at temperatures down to 0.5 K with high-magnetic pulsed-fields, we observe a crossover from two-dimensional to three-dimensional superconducting states which can be manipulated by the ionic size fluctuations in the rare-earth spacer layer. Such a large degree of controllability is desired for tailoring strongly two/three-dimensional superconductors and navigating various pairing landscapes for a better understanding of the correlation between reduced dimensionality and unconventional pairing. These results illuminate new directions to unravel the high-temperature superconducting pairing mechanism.
Comment: 30 pages, 4 main figures, 8 extended data figures
نوع الوثيقة: Working Paper
URL الوصول: http://arxiv.org/abs/2301.07606
رقم الأكسشن: edsarx.2301.07606
قاعدة البيانات: arXiv