Infrared-induced ultrafast melting of nanostructured platinum films probed by an X-ray free-electron laser

التفاصيل البيبلوغرافية
العنوان: Infrared-induced ultrafast melting of nanostructured platinum films probed by an X-ray free-electron laser
المؤلفون: Gelisio, Luca, Kim, Young Yong, Lim, Seon Woo, Nam, Daewoong, Eom, Intae, Kim, Minseok, Kim, Sangsoo, Khubbutdinov, Ruslan, Xiang, Li, Lee, Hoyeol, Ree, Moonhor, Kim, Chae Un, Vartanyants, Ivan A.
سنة النشر: 2023
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Materials Science
الوصف: Understanding melting in metals is a hot topic of present research. This may be accomplished by pumping the system with infrared (IR) laser radiation, and probing it with hard X-rays produced by an X-ray Free-Electron Laser (XFEL). In this work we studied nanostructured polycrystalline thin films of platinum that were illuminated by IR radiation of increasing fluences. We characterized the structural response as well as the nucleation and propagation of the liquid phase as a function of time delay between the IR pump and X-ray probe. We observed partial melting of the samples for IR fluences higher than 200 mJ$\cdot$cm$^{-2}$. To fit the contribution of the liquid phase to the scattering pattern in platinum we applied a model of liquid metal. The two-temperature model simulations were performed to understand the solid-state fraction of the sample heating process as a function of time delay and fluence.
نوع الوثيقة: Working Paper
URL الوصول: http://arxiv.org/abs/2302.12362
رقم الأكسشن: edsarx.2302.12362
قاعدة البيانات: arXiv