Light-to-heat conversion of optically trapped hot Brownian particles

التفاصيل البيبلوغرافية
العنوان: Light-to-heat conversion of optically trapped hot Brownian particles
المؤلفون: Ortiz-Rivero, Elisa, Orozco-Barrera, Sergio, Chatterjee, Hirak, Gonzalez-Gomez, Carlos D., Caro, Carlos, Garcia-Martin, Maria L., Haro-Gonzalez, Patricia, Rica, Raul A., Gamez, Francisco
المصدر: ACS Nano 2024
سنة النشر: 2023
المجموعة: Condensed Matter
Physics (Other)
مصطلحات موضوعية: Condensed Matter - Mesoscale and Nanoscale Physics, Physics - Applied Physics
الوصف: Anisotropic hybrid nanostructures stand out as promising therapeutic agents in photothermal conversion-based treatments. Accordingly, understanding local heat generation mediated by light-to-heat conversion of absorbing multicomponent nanoparticles at the single particle level have both forthwith become a subject of broad and current interest. Nonetheless, evaluating reliable temperature profiles around a single trapped nanoparticle is challenging from all experimental, computational, and fundamental viewpoints. Committed to filling this gap, the heat generation of an anisotropic hybrid nanostructure is explored by means of two different experimental approaches from which the local temperature is measured in a direct or indirect way, all in the context of the hot Brownian motion theory. The results were compared with analytical results supported by the numerical computation of the wavelength-dependent absorption efficiencies in the discrete dipole approximation for scattering calculations, which has been here extended to inhomogeneous nanostructures. Overall, we provide a consistent and comprehensive view of the heat generation in optical traps of highly absorbing particles under the viewpoint of the hot Brownian motion theory.
نوع الوثيقة: Working Paper
DOI: 10.1021/acsnano.3c07086
URL الوصول: http://arxiv.org/abs/2309.11866
رقم الأكسشن: edsarx.2309.11866
قاعدة البيانات: arXiv