Field-induced quantum phase in a frustrated zigzag-square lattice

التفاصيل البيبلوغرافية
العنوان: Field-induced quantum phase in a frustrated zigzag-square lattice
المؤلفون: Yamaguchi, Hironori, Shimamura, Kazutoshi, Yoshida, Yasuo, Matsuo, Akira, Kindo, Koichi, Nakano, Kiichi, Morota, Satoshi, Hosokoshi, Yuko, Kida, Takanori, Iwasaki, Yoshiki, Shimono, Seiya, Araki, Koji, Hagiwara, Masayuki
المصدر: Phys. Rev. Mater. 7, L091401 (2023)
سنة النشر: 2023
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons
الوصف: This study presents the experimental realization of a spin-1/2 zigzag-square lattice in a verdazyl-based complex, namely ($m$-Py-V-2,6-F$_2$)$[$Cu(hfac)$_2]$. Molecular orbital calculations suggest the presence of five types of frustrated exchange couplings. Our observations reveal an incremental increase in the magnetization curve beyond a critical field, signifying a phase transition from the antiferromagnetic ordered state to a quantum state characterized by a 1/2 plateau. This intriguing behavior arises from the effective stabilization of a zigzag chain by the external fields. These results provide evidence for field-induced dimensional reduction in a zigzag-square lattice attributed to the effects of frustration.
Comment: 5 pages, 4 figures
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevMaterials.7.L091401
URL الوصول: http://arxiv.org/abs/2309.14619
رقم الأكسشن: edsarx.2309.14619
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevMaterials.7.L091401