Spin-Phonon Coupling in Transition Metal Insulators II: Spin-Orbital Moments, Chiral Phonons and Application to $\alpha$-RuCl$_3$

التفاصيل البيبلوغرافية
العنوان: Spin-Phonon Coupling in Transition Metal Insulators II: Spin-Orbital Moments, Chiral Phonons and Application to $\alpha$-RuCl$_3$
المؤلفون: Dhakal, Ramesh, Kaib, David A. S., Biswas, Sananda, Valenti, Roser, Winter, Stephen M.
سنة النشر: 2024
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons
الوصف: We apply a recently developed first-principles based approach for treating generic spin-phonon couplings in materials with strong spin-orbit coupling to study $\alpha$-RuCl$_3$. Of particular focus is the potential for this material to exhibit a phonon thermal Hall effect induced by spin-phonon interactions. We find that spin-orbit coupling significantly enriches the form of these interactions, and imbues them with chirality that is conducive to generating finite phonon Berry curvatures. We show that this leads to a phonon thermal Hall effect that qualitatively reproduces the measured field dependence of $\kappa_{xy}$ without requiring a field-induced spin liquid.
Comment: 20 pages, 9 figures including supplemental material
نوع الوثيقة: Working Paper
URL الوصول: http://arxiv.org/abs/2407.00660
رقم الأكسشن: edsarx.2407.00660
قاعدة البيانات: arXiv