Two-dimensional Topological Ferroelectric Metal with Giant Ghift Current

التفاصيل البيبلوغرافية
العنوان: Two-dimensional Topological Ferroelectric Metal with Giant Ghift Current
المؤلفون: Yang, Liu, Li, Lei, Yu, Zhi-Ming, Wu, Menghao, Yao, Yugui
سنة النشر: 2024
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Materials Science, Condensed Matter - Mesoscale and Nanoscale Physics
الوصف: The pursuit for "ferroelectric metal" which combines seemingly incompatible spontaneous electric polarization and metallicity, has been assiduously ongoing but remains elusive. Unlike traditional ferroelectrics with a wide band gap, ferroelectric (FE) metals can naturally incorporate nontrivial band topology near the Fermi level, endowing them with additional exotic properties. Here, we show first-principles evidence that the metallic PtBi2 monolayer is an intrinsic two-dimensional (2D) topological FE metal, characterized by out-of-plane polarization and a moderate switching barrier. Moreover, it exhibits a topologically nontrivial electronic structure with Z2 invariant equal to 1, leading to a significant FE bulk photovoltaic effect. A slight strain can further enhance this effect to a remarkable level, which far surpass that of previously reported 2D/3D FE materials. Our work provides an important step towards realizing intrinsic monolayer topological FE metals and paves a promising way for future nonlinear optical devices.
Comment: 7 pages, 5 figures
نوع الوثيقة: Working Paper
URL الوصول: http://arxiv.org/abs/2408.01982
رقم الأكسشن: edsarx.2408.01982
قاعدة البيانات: arXiv