دورية أكاديمية

Weakly-Correlated Nature of Ferromagnetism in Nonsymmorphic CrO_{2} Revealed by Bulk-Sensitive Soft-X-Ray ARPES

التفاصيل البيبلوغرافية
العنوان: Weakly-Correlated Nature of Ferromagnetism in Nonsymmorphic CrO_{2} Revealed by Bulk-Sensitive Soft-X-Ray ARPES
المؤلفون: F. Bisti, V. A. Rogalev, M. Karolak, S. Paul, A. Gupta, T. Schmitt, G. Güntherodt, V. Eyert, G. Sangiovanni, G. Profeta, V. N. Strocov
المصدر: Physical Review X, Vol 7, Iss 4, p 041067 (2017)
بيانات النشر: American Physical Society, 2017.
سنة النشر: 2017
المجموعة: LCC:Physics
مصطلحات موضوعية: Physics, QC1-999
الوصف: Chromium dioxide CrO_{2} belongs to a class of materials called ferromagnetic half-metals, whose peculiar aspect is that they act as a metal in one spin orientation and as a semiconductor or insulator in the opposite one. Despite numerous experimental and theoretical studies motivated by technologically important applications of this material in spintronics, its fundamental properties such as momentum-resolved electron dispersions and the Fermi surface have so far remained experimentally inaccessible because of metastability of its surface, which instantly reduces to amorphous Cr_{2}O_{3}. In this work, we demonstrate that direct access to the native electronic structure of CrO_{2} can be achieved with soft-x-ray angle-resolved photoemission spectroscopy whose large probing depth penetrates through the Cr_{2}O_{3} layer. For the first time, the electronic dispersions and Fermi surface of CrO_{2} are measured, which are fundamental prerequisites to solve the long debate on the nature of electronic correlations in this material. Since density functional theory augmented by a relatively weak local Coulomb repulsion gives an exhaustive description of our spectroscopic data, we rule out strong-coupling theories of CrO_{2}. Crucial for the correct interpretation of our experimental data in terms of the valence-band dispersions is the understanding of a nontrivial spectral response of CrO_{2} caused by interference effects in the photoemission process originating from the nonsymmorphic space group of the rutile crystal structure of CrO_{2}.
نوع الوثيقة: article
وصف الملف: electronic resource
اللغة: English
تدمد: 2160-3308
Relation: https://doaj.org/toc/2160-3308
DOI: 10.1103/PhysRevX.7.041067
URL الوصول: https://doaj.org/article/05bd714a7d994efcbc6748f27da5697a
رقم الأكسشن: edsdoj.05bd714a7d994efcbc6748f27da5697a
قاعدة البيانات: Directory of Open Access Journals
الوصف
تدمد:21603308
DOI:10.1103/PhysRevX.7.041067