دورية أكاديمية

Optical cycling of AlF molecules

التفاصيل البيبلوغرافية
العنوان: Optical cycling of AlF molecules
المؤلفون: S Hofsäss, M Doppelbauer, S C Wright, S Kray, B G Sartakov, J Pérez-Ríos, G Meijer, S Truppe
المصدر: New Journal of Physics, Vol 23, Iss 7, p 075001 (2021)
بيانات النشر: IOP Publishing, 2021.
سنة النشر: 2021
المجموعة: LCC:Science
LCC:Physics
مصطلحات موضوعية: laser cooling, cold molecules, buffer gas cooling, Science, Physics, QC1-999
الوصف: Aluminium monofluoride (AlF) is a promising candidate for laser cooling and trapping at high densities. We show efficient production of AlF in a bright, pulsed cryogenic buffer gas beam, and demonstrate rapid optical cycling on the Q rotational lines of the A ^1 Π ↔ X ^1 Σ ^+ transition. We measure the brightness of the molecular beam to be >10 ^12 molecules per steradian per pulse in a single rotational state and present a new method to determine its velocity distribution in a single shot. The photon scattering rate of the optical cycling scheme is measured using three different methods, and is compared to theoretical predictions of the optical Bloch equations and a simplified rate equation model. Despite the large number of Zeeman sublevels (up to 216 for the Q(4) transition) involved, a high scattering rate of at least 17(2) × 10 ^6 s ^−1 can be sustained using a single, fixed-frequency laser without the need to modulate the polarisation. We deflect the molecu-lar beam using the radiation pressure force and measure an acceleration of 8.7(1.5) × 10 ^5 m s ^−2 . Losses from the optical cycle due to vibrational branching to X ^1 Σ ^+ , v ″ = 1 are addressed efficiently with a single repump laser. Further, we investigate two other loss channels, parity mixing by stray electric fields and photo-ionisation. The upper bounds for these effects are sufficiently low to allow loading into a magneto‐optical trap.
نوع الوثيقة: article
وصف الملف: electronic resource
اللغة: English
تدمد: 1367-2630
Relation: https://doaj.org/toc/1367-2630
DOI: 10.1088/1367-2630/ac06e5
URL الوصول: https://doaj.org/article/0977be5e9c814309b3b96ec99e603487
رقم الأكسشن: edsdoj.0977be5e9c814309b3b96ec99e603487
قاعدة البيانات: Directory of Open Access Journals
الوصف
تدمد:13672630
DOI:10.1088/1367-2630/ac06e5