دورية أكاديمية

Exchange-bias and magnetic anisotropy fields in core–shell ferrite nanoparticles

التفاصيل البيبلوغرافية
العنوان: Exchange-bias and magnetic anisotropy fields in core–shell ferrite nanoparticles
المؤلفون: F. G. Silva, J. Depeyrot, Yu. L. Raikher, V. I. Stepanov, I. S. Poperechny, R. Aquino, G. Ballon, J. Geshev, E. Dubois, R. Perzynski
المصدر: Scientific Reports, Vol 11, Iss 1, Pp 1-10 (2021)
بيانات النشر: Nature Portfolio, 2021.
سنة النشر: 2021
المجموعة: LCC:Medicine
LCC:Science
مصطلحات موضوعية: Medicine, Science
الوصف: Abstract Exchange bias properties of MnFe $$_2$$ 2 O $$_4$$ 4 @ $$\gamma$$ γ –Fe $$_2$$ 2 O $$_3$$ 3 core–shell nanoparticles are investigated. The measured field and temperature dependencies of the magnetization point out a well-ordered ferrimagnetic core surrounded by a layer with spin glass-like arrangement. Quasi-static SQUID magnetization measurements are presented along with high-amplitude pulse ones and are cross-analyzed by comparison against ferromagnetic resonance experiments at 9 GHz. These measurements allow one to discern three types of magnetic anisotropies affecting the dynamics of the magnetic moment of the well-ordered ferrimagnetic NP’s core viz. the easy-axis (uniaxial) anisotropy, the unidirectional exchange-bias anisotropy and the rotatable anisotropy. The uniaxial anisotropy originates from the structural core–shell interface. The unidirectional exchange-bias anisotropy is associated with the spin-coupling at the ferrimagnetic/spin glass-like interface; it is observable only at low temperatures after a field-cooling process. The rotatable anisotropy is caused by partially-pinned spins at the core/shell interface; it manifests itself as an intrinsic field always parallel to the external applied magnetic field. The whole set of experimental results is interpreted in the framework of superparamagnetic theory, i.e., essentially taking into account the effect of thermal fluctuations on the magnetic moment of the particle core. In particular, it is found that the rotatable anisotropy of our system is of a uniaxial type.
نوع الوثيقة: article
وصف الملف: electronic resource
اللغة: English
تدمد: 2045-2322
Relation: https://doaj.org/toc/2045-2322
DOI: 10.1038/s41598-021-84843-0
URL الوصول: https://doaj.org/article/0b4b3c17e92d4ce8b37a22ea8f81edf1
رقم الأكسشن: edsdoj.0b4b3c17e92d4ce8b37a22ea8f81edf1
قاعدة البيانات: Directory of Open Access Journals
الوصف
تدمد:20452322
DOI:10.1038/s41598-021-84843-0