دورية أكاديمية

Strain-induced specific orbital control in a Heusler alloy-based interfacial multiferroics

التفاصيل البيبلوغرافية
العنوان: Strain-induced specific orbital control in a Heusler alloy-based interfacial multiferroics
المؤلفون: Jun Okabayashi, Takamasa Usami, Amran Mahfudh Yatmeidhy, Yuichi Murakami, Yu Shiratsuchi, Ryoichi Nakatani, Yoshihiro Gohda, Kohei Hamaya
المصدر: NPG Asia Materials, Vol 16, Iss 1, Pp 1-10 (2024)
بيانات النشر: Nature Portfolio, 2024.
سنة النشر: 2024
المجموعة: LCC:Materials of engineering and construction. Mechanics of materials
LCC:Biotechnology
مصطلحات موضوعية: Materials of engineering and construction. Mechanics of materials, TA401-492, Biotechnology, TP248.13-248.65
الوصف: Abstract For the development of spintronic devices, the control of magnetization by a low electric field is necessary. The microscopic origin of manipulating spins relies on the control of orbital magnetic moments (m orb) by strain; this is essential for the high performance magnetoelectric (ME) effect. Herein, electric-field induced X-ray magnetic circular dichroism (XMCD) is used to determine the changes in m orb by piezoelectric strain and clarify the relationship between the strain and m orb in an interfacial multiferroics system with a significant ME effect; the system consists of the Heusler alloy Co2FeSi on a ferroelectric Pb(Mg1/3Nb2/3)O3-PbTiO3 substrate. Element-specific investigations of the orbital states by operando XMCD and the local environment via extended X-ray absorption fine structure (EXAFS) analysis show that the modulation of only the Fe sites in Co2FeSi primarily contributes to the giant ME effect. The density functional theory calculations corroborate this finding, and the growth of the high index (422) plane in Co2FeSi results in a giant ME effect. These findings elucidate the element-specific orbital control using reversible strain, called the ‘orbital elastic effect,’ and can provide guidelines for material designs with a giant ME effect.
نوع الوثيقة: article
وصف الملف: electronic resource
اللغة: English
تدمد: 1884-4057
Relation: https://doaj.org/toc/1884-4057
DOI: 10.1038/s41427-023-00524-6
URL الوصول: https://doaj.org/article/3c3ef83f7d2843faad8ee83808e06a42
رقم الأكسشن: edsdoj.3c3ef83f7d2843faad8ee83808e06a42
قاعدة البيانات: Directory of Open Access Journals
الوصف
تدمد:18844057
DOI:10.1038/s41427-023-00524-6