دورية أكاديمية

Excitonic Linewidth Approaching the Homogeneous Limit in MoS_{2}-Based van der Waals Heterostructures

التفاصيل البيبلوغرافية
العنوان: Excitonic Linewidth Approaching the Homogeneous Limit in MoS_{2}-Based van der Waals Heterostructures
المؤلفون: F. Cadiz, E. Courtade, C. Robert, G. Wang, Y. Shen, H. Cai, T. Taniguchi, K. Watanabe, H. Carrere, D. Lagarde, M. Manca, T. Amand, P. Renucci, S. Tongay, X. Marie, B. Urbaszek
المصدر: Physical Review X, Vol 7, Iss 2, p 021026 (2017)
بيانات النشر: American Physical Society, 2017.
سنة النشر: 2017
المجموعة: LCC:Physics
مصطلحات موضوعية: Physics, QC1-999
الوصف: The strong light-matter interaction and the valley selective optical selection rules make monolayer (ML) MoS_{2} an exciting 2D material for fundamental physics and optoelectronics applications. But, so far, optical transition linewidths even at low temperature are typically as large as a few tens of meV and contain homogeneous and inhomogeneous contributions. This prevented in-depth studies, in contrast to the better-characterized ML materials MoSe_{2} and WSe_{2}. In this work, we show that encapsulation of ML MoS_{2} in hexagonal boron nitride can efficiently suppress the inhomogeneous contribution to the exciton linewidth, as we measure in photoluminescence and reflectivity a FWHM down to 2 meV at T=4 K. Narrow optical transition linewidths are also observed in encapsulated WS_{2}, WSe_{2}, and MoSe_{2} MLs. This indicates that surface protection and substrate flatness are key ingredients for obtaining stable, high-quality samples. Among the new possibilities offered by the well-defined optical transitions, we measure the homogeneous broadening induced by the interaction with phonons in temperature-dependent experiments. We uncover new information on spin and valley physics and present the rotation of valley coherence in applied magnetic fields perpendicular to the ML.
نوع الوثيقة: article
وصف الملف: electronic resource
اللغة: English
تدمد: 2160-3308
Relation: https://doaj.org/toc/2160-3308
DOI: 10.1103/PhysRevX.7.021026
URL الوصول: https://doaj.org/article/45bc5bbfd1d949fca67aef7e4b15dcb1
رقم الأكسشن: edsdoj.45bc5bbfd1d949fca67aef7e4b15dcb1
قاعدة البيانات: Directory of Open Access Journals
الوصف
تدمد:21603308
DOI:10.1103/PhysRevX.7.021026