دورية أكاديمية
Influence of Oxidative Properties of CexZr1−xO2 Catalyst on Partial Oxidation of Dimethyl Ether
العنوان: | Influence of Oxidative Properties of CexZr1−xO2 Catalyst on Partial Oxidation of Dimethyl Ether |
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المؤلفون: | Zhu Fu, Ping Qi, Huimin Liu, Qijian Zhang, Yonghua Zhao, Xiaoqian Feng |
المصدر: | Catalysts, Vol 12, Iss 12, p 1536 (2022) |
بيانات النشر: | MDPI AG, 2022. |
سنة النشر: | 2022 |
المجموعة: | LCC:Chemical technology LCC:Chemistry |
مصطلحات موضوعية: | DME, partial oxidation, hydrogen production, CexZr1−xO2, Chemical technology, TP1-1185, Chemistry, QD1-999 |
الوصف: | Partial oxidation of dimethyl ether (DME) to hydrogen is an efficient route for hydrogen production for application in SOFC. However, quite a large amount of CO2 as a byproduct has been an important obstacle. In this work, cerium–zirconium solid solution (CexZr1−xO2) was applied to determine how the oxidative properties of the catalyst affect the production of CO2 in the partial oxidation of DME. The results show that the catalyst with more adsorbed oxygen (Oads) rather than the lattice oxygen has stronger oxidizability and gives higher DME conversion as well as higher CO2 yield, due to the overoxidation of CO. |
نوع الوثيقة: | article |
وصف الملف: | electronic resource |
اللغة: | English |
تدمد: | 2073-4344 |
Relation: | https://www.mdpi.com/2073-4344/12/12/1536; https://doaj.org/toc/2073-4344 |
DOI: | 10.3390/catal12121536 |
URL الوصول: | https://doaj.org/article/55265399a7ed4e06bd517eb04b6f2bd2 |
رقم الأكسشن: | edsdoj.55265399a7ed4e06bd517eb04b6f2bd2 |
قاعدة البيانات: | Directory of Open Access Journals |
تدمد: | 20734344 |
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DOI: | 10.3390/catal12121536 |