Advances in X-ray laser sources have paved the way to relativistic attosecond X-ray laser pulses and opened up the possibility of exploring high-energy-density physics with this technology. With particle-in-cell simulations, we investigate the interaction of realistic metal crystals with relativistic X-ray laser pulses of parameters that will be available in the near future. A wakefield of the order of TV/cm is excited in the crystal and accelerates trapped electrons stably even though the wakefield is locally modulated by the crystal lattice. Electron injection either occurs at the sharp crystal–vacuum boundary or is controlled by coating the crystal with a high-density film. High-repetition-rate attosecond (20 as) monoenergetic electron beams of energy 125 MeV, charge 100 fC, and emittance 1.6 × 10−9 m rad can be produced by shining MHz X-ray laser pulses of energy 2.1 mJ onto coated crystals several micrometers thick. Such a miniature crystal accelerator, which has high reproducibility and allows sufficient control of the parameters of the electron beams, greatly expands the applications of X-ray free electron lasers. For example, it could serve as an ideal electron source for ultrafast electron diffraction and ultrafast electron microscopy to achieve attosecond resolution.
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