دورية أكاديمية

An 800-year high-resolution black carbon ice core record from Lomonosovfonna, Svalbard

التفاصيل البيبلوغرافية
العنوان: An 800-year high-resolution black carbon ice core record from Lomonosovfonna, Svalbard
المؤلفون: D. Osmont, I. A. Wendl, L. Schmidely, M. Sigl, C. P. Vega, E. Isaksson, M. Schwikowski
المصدر: Atmospheric Chemistry and Physics, Vol 18, Pp 12777-12795 (2018)
بيانات النشر: Copernicus Publications, 2018.
سنة النشر: 2018
المجموعة: LCC:Physics
LCC:Chemistry
مصطلحات موضوعية: Physics, QC1-999, Chemistry, QD1-999
الوصف: Produced by the incomplete combustion of fossil fuel and biomass, black carbon (BC) contributes to Arctic warming by reducing snow albedo and thus triggering a snow-albedo feedback leading to increased snowmelt. Therefore, it is of high importance to assess past BC emissions to better understand and constrain their role. However, only a few long-term BC records are available from the Arctic, mainly originating from Greenland ice cores. Here, we present the first long-term and high-resolution refractory black carbon (rBC) record from Svalbard, derived from the analysis of two ice cores drilled at the Lomonosovfonna ice field in 2009 (LF-09) and 2011 (LF-11) and covering 800 years of atmospheric emissions. Our results show that rBC concentrations strongly increased from 1860 on due to anthropogenic emissions and reached two maxima, at the end of the 19th century and in the middle of the 20th century. No increase in rBC concentrations during the last decades was observed, which is corroborated by atmospheric measurements elsewhere in the Arctic but contradicts a previous study from another ice core from Svalbard. While melting may affect BC concentrations during periods of high temperatures, rBC concentrations remain well preserved prior to the 20th century due to lower temperatures inducing little melt. Therefore, the preindustrial rBC record (before 1800), along with ammonium (NH4+), formate (HCOO−) and specific organic markers (vanillic acid, VA, and p-hydroxybenzoic acid, p-HBA), was used as a proxy for biomass burning. Despite numerous single events, no long-term trend was observed over the time period 1222–1800 for rBC and NH4+. In contrast, formate, VA, and p-HBA experience multi-decadal peaks reflecting periods of enhanced biomass burning. Most of the background variations and single peak events are corroborated by other ice core records from Greenland and Siberia. We suggest that the paleofire record from the LF ice core primarily reflects biomass burning episodes from northern Eurasia, induced by decadal-scale climatic variations.
نوع الوثيقة: article
وصف الملف: electronic resource
اللغة: English
تدمد: 1680-7316
1680-7324
Relation: https://www.atmos-chem-phys.net/18/12777/2018/acp-18-12777-2018.pdf; https://doaj.org/toc/1680-7316; https://doaj.org/toc/1680-7324
DOI: 10.5194/acp-18-12777-2018
URL الوصول: https://doaj.org/article/8ac9a806130d4c1fae6680fcf9e2f647
رقم الأكسشن: edsdoj.8ac9a806130d4c1fae6680fcf9e2f647
قاعدة البيانات: Directory of Open Access Journals
الوصف
تدمد:16807316
16807324
DOI:10.5194/acp-18-12777-2018