دورية أكاديمية
Atomic Dispersed Hetero-Pairs for Enhanced Electrocatalytic CO2 Reduction
العنوان: | Atomic Dispersed Hetero-Pairs for Enhanced Electrocatalytic CO2 Reduction |
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المؤلفون: | Zhaoyong Jin, Meiqi Yang, Yilong Dong, Xingcheng Ma, Ying Wang, Jiandong Wu, Jinchang Fan, Dewen Wang, Rongshen Xi, Xiao Zhao, Tianyi Xu, Jingxiang Zhao, Lei Zhang, David J. Singh, Weitao Zheng, Xiaoqiang Cui |
المصدر: | Nano-Micro Letters, Vol 16, Iss 1, Pp 1-13 (2023) |
بيانات النشر: | SpringerOpen, 2023. |
سنة النشر: | 2023 |
المجموعة: | LCC:Technology |
مصطلحات موضوعية: | CO2 reduction reaction, Atomic dispersed catalyst, Hetero-diatomic pair, Ad-desorption energy, Linear scaling relation, Technology |
الوصف: | Highlights A unique atomic dispersed hetero-pair was successfully synthesized, consisting of Mo-Fe di-atoms anchored on N-doped carbon carrier. This strategy breaks the linear scaling relationships of electrocatalytic CO2 reduction by simultaneously regulating the *COOH adsorption energy and *CO desorption energy. The as-prepared MoFe–N–C exhibits excellent performance for CO2RR to CO with a high turnover frequency (TOF) of 3336.21 h−1, CO Faradaic efficiency (FECO) of 95.96% at − 0.60 V (versus RHE) and outstanding stability. |
نوع الوثيقة: | article |
وصف الملف: | electronic resource |
اللغة: | English |
تدمد: | 2311-6706 2150-5551 |
Relation: | https://doaj.org/toc/2311-6706; https://doaj.org/toc/2150-5551 |
DOI: | 10.1007/s40820-023-01214-2 |
URL الوصول: | https://doaj.org/article/985533e6099d4305b5666cc0c34a87bd |
رقم الأكسشن: | edsdoj.985533e6099d4305b5666cc0c34a87bd |
قاعدة البيانات: | Directory of Open Access Journals |
تدمد: | 23116706 21505551 |
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DOI: | 10.1007/s40820-023-01214-2 |